1,728 research outputs found
Phase Diagram of -(BEDT-TTF)ICl under High Pressure Based on the First-Principles Electronic Structure
We present a theoretical study on the superconductivity of
-(BEDT-TTF)ICl at 14.2 K under a high hydrostatic
pressure recently found, which is the highest among organic superconductors. In
the present work, we study an effective model using the fluctuation-exchange
(FLEX) approximation based on the results of first-principles calculation. In
the obtained phase diagram, the superconductivity with -like symmetry
is realized next to the antiferromagnetic phase, as a result of the
one-dimensional to two-dimensional crossover driven by the pressure.Comment: 4 pages, 3 figures. accepted for publication in J. Phys. Soc. Jpn.
errors correcte
Two-band Fluctuation Exchange Study on the Superconductivity of -(BEDT-TTF)ICl under High Pressure
We study the pressure dependence of the superconducting transition
temperature of an organic superconductor -(BEDT-TTF)ICl by
applying the fluctuation exchange method to the Hubbard model on the original
two-band lattice at 3/4-filling rather than the single band model in the strong
dimerization limit. Our study is motivated by the fact that hopping parameters
evaluated from a first-principles study suggest that the dimerization of the
BEDT-TTF molecules is not so strong especially at high pressure. Solving the
linearized Eliashberg's equation, a d-wave-like superconducting state
with realistic values of is obtained in a pressure regime somewhat higher
than the actual experimental result. These results are similar to those
obtained within the single band model in the previous study by Kino {\it et
al}. We conclude that the resemblance to the dimer limit is due to a
combination of a good Fermi surface nesting, a large density of states near the
Fermi level, and a moderate dimerization, which cooperatively enhance electron
correlation effects and also the superconducting .Comment: 6 pages, 8 figure
Charge Ordering in Organic ET Compounds
The charge ordering phenomena in quasi two-dimensional 1/4-filled organic
compounds (ET)_2X (ET=BEDT-TTF) are investigated theoretically for the
and -type structures, based on the Hartree approximation for the
extended Hubbard models with both on-site and intersite Coulomb interactions.
It is found that charge ordered states of stripe-type are stabilized for the
relevant values of Coulomb energies, while the spatial pattern of the stripes
sensitively depends on the anisotropy of the models. By comparing the results
of calculations with the experimental facts, where the effects of quantum
fluctuation is incorporated by mapping the stripe-type charge ordered states to
the S=1/2 Heisenberg Hamiltonians, the actual charge patterns in the insulating
phases of -(ET)_2MM'(SCN)_4 and -(ET)_2I_3 are deduced.
Furthermore, to obtain a unified view among the , and
-(ET)_2X families, the stability of the charge ordered state in
competition with the dimeric antiferromagnetic state viewed as the Mott
insulating state, which is typically realized in -type compounds, and
with the paramagnetic metallic state, is also pursued by extracting essential
parameters.Comment: 35 pages, 27 figures, submitted to J. Phys. Soc. Jp
Gossamer Superconductivity near Antiferromagnetic Mott Insulator in Layered Organic Conductors
Layered organic superconductors are on the verge of the Mott insulator. We
use Gutzwiller variational method to study a Hubbard model including a spin
exchange coupling term. The ground state is found to be a Gossamer
superconductor at small on-site Coulomb repulsion U and an antiferromagnetic
Mott insulator at large U, separated by a first order phase transition. Our
theory is qualitatively consistent with major experiments reported in organic
superconductors.Comment: 5 pages, 3 figure
Charge Ordering in alpha-(BEDT-TTF)2I3 by synchrotron x-ray diffraction
The spatial charge arrangement of a typical quasi-two-dimensional organic
conductor alpha-(BEDT-TTF)2I3 is revealed by single crystal structure analysis
using synchrotron radiation. The results show that the horizontal stripe type
structure, which was suggested by mean field theory, is established. We also
find the charge disproportion above the metal-insulator transition temperature
and a significant change in transfer integrals caused by the phase transition.
Our result elucidates the insulating phase of this material as a 2k_F charge
density localization.Comment: 8 pages, 5 figures, 1 tabl
Antiferromagnetic Phases of One-Dimensional Quarter-Filled Organic Conductors
The magnetic structure of antiferromagnetically ordered phases of
quasi-one-dimensional organic conductors is studied theoretically at absolute
zero based on the mean field approximation to the quarter-filled band with
on-site and nearest-neighbor Coulomb interaction. The differences in magnetic
properties between the antiferromagnetic phase of (TMTTF)X and the spin
density wave phase in (TMTSF)X are seen to be due to a varying degrees of
roles played by the on-site Coulomb interaction. The nearest-neighbor Coulomb
interaction introduces charge disproportionation, which has the same spatial
periodicity as the Wigner crystal, accompanied by a modified antiferromagnetic
phase. This is in accordance with the results of experiments on (TMTTF)Br
and (TMTTF)SCN. Moreover, the antiferromagnetic phase of (DI-DCNQI)Ag
is predicted to have a similar antiferromagnetic spin structure.Comment: 8 pages, LaTeX, 4 figures, uses jpsj.sty, to be published in J. Phys.
Soc. Jpn. 66 No. 5 (1997
Ultrasonic Imaging Systems
The use of ultrasonic imaging systems for non-destructive evaluation is increasing, with particular interest being paid to research into real time and quasi-real time imaging systems. Photos are shown which were taken using an electronically scanned and focused real time ultrasonic imaging system. The system can be operated with longitudinal waves, shear waves, Rayleigh waves, and lamb waves in the 1.5 MHz to 3.5 MHz frequency range, and has been successfully used on composite materials (boron fiber epoxy on titanium) and on a number of metals (steel, aluminum, and titanium). This system has been operated in both transmission and reflection modes; examples of each are shown
Magnetic-Field-Induced Antiferromagnetism in Two-Dimensional Hubbard Model: Analysis of CeRhIn
We propose the mechanism for the magnetic-field-induced antiferromagnetic
(AFM) state in a two-dimensional Hubbard model in the vicinity of the AFM
quantum critical point (QCP), using the fluctuation-exchange (FLEX)
approximation by taking the Zeeman energy due to the magnetic field into
account. In the vicinity of the QCP, we find that the AFM correlation
perpendicular to is enhanced, whereas that parallel to is reduced. This
fact means that the finite magnetic field increases , with the AFM order
perpendicular to . The increment in can be understood in terms of the
reduction of both quantum and thermal fluctuations due to the magnetic field,
which is caused by the self-energy effect within the FLEX approximation. The
present study naturally explains the increment in in CeRhIn_5 under the
magnetic field found recently.Comment: 5 page
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